I already have Raphael marked as the Seraph of Love, I meant more of what he would do other than rule the 4th Heaven. For instance, Uriel is in charge of the army and Jophiel is in charge of espionage and knowledge. I also need a virtue for Zadkiel (Not necessarily one of the Seven Heavenly Virtues).
As for other Good outsiders, I always though Oberon and Titania should be the leaders of the CG outsiders. Still, we've got enough going on with LG; we should probably hold off on the other alignments.